By Volkmar Dierolf
This e-book bargains with the mutual interplay and effort move among digital illness states of F facilities and disorder ions (e.g. infrequent earth parts) and neighbouring molecular defects (OH-, CN-) in alkali halides. those version disorder structures convey a truly exciting and ambiguous personality simply because they behave like remoted defects in a single example yet like supermolecules in others. The textual content supplies an outline of the subject and discusses attainable functions. It covers a variety of spectroscopic tools utilized to the platforms and studies numerous techniques for his or her theoretical interpretation. It comprises greater than a hundred illustrations, figures and tables in addition to many formerly unpublished effects. This ebook offers a necessary source for additional experiences into this and comparable fields.
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Additional info for Electronic Defect States in Alkali Halides: Effects of Interaction with Molecular Ions
52, 6272 (1970). 40 25. C. Manneback, Physica 17, 1001 (1951). 40 26. C. W. Struck and W. H. Fonger, J. Lumin. 10, 1 (1975). 40, 45 27. C. W. Struck and W. H. Fonger, J. Lumin. 14, 253 (1976). 40, 45 28. R. Wallace, Chem. Phys. Lett. 37, 115 (1976). 41 29. M. Sage, Chem. Phys. 35, 375 (1978). 41 30. D. D. thesis, Universit¨ at GH Paderborn, 1997. 41 References 31. 32. 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. 44. 45. 49 J. West, S. H. Lin, and K. T. Tsen, J. Chem. Phys. 99, 7574 (1993). 42 J.
8) remain valid within a ﬁrst-order approximation and we can replace ψe,g by ψg and ψe . Written in that way, the transition matrix element describes a transition of the molecule under simultaneous change of the electronic state. In a series of papers, Struck and Fonger [26, 27, 40, 41] have shown that the corresponding matrix elements and their thermal averages can be related to each other by recursion formulas. To give an example un |ξ| vm = ≈ 1 m · un | vm−1 + 2 1 m · un | vm−1 . 18) and that a change in anharmonicity and vibrational coupling strength will inﬂuence all of them.
Wood, Phys. Rev. 123, 766 (1961). 17 31. G. Baldini and M. Guzzi, Phys. Status Solidi 30, 601 (1968). 17 32. E. Mulazzi, G. F. Nardelli, and N. Terzi, Phys. Rev. 172, 847 (1968). 17 33. V. Dierolf, Phys. Rev. B 60, 12601 (1999). 17 34. A. J. Ramponi and J. C. Wright, Phys. Rev. B 35, 2413 (1987). 18 3 Properties of Molecular Defects Molecular defects are commonly described as anharmonic oscillators, the basic properties of which have been well studied for a long time  and most aspects have been treated in textbooks .
Electronic Defect States in Alkali Halides: Effects of Interaction with Molecular Ions by Volkmar Dierolf